Giri, Bishnubasu’s team published research in Inorganica Chimica Acta in 2020-03-01 | CAS: 100-70-9

Inorganica Chimica Acta published new progress about Crystal structure. 100-70-9 belongs to class nitriles-buliding-blocks, name is Picolinonitrile, and the molecular formula is C6H4N2, Product Details of C6H4N2.

Giri, Bishnubasu published the artcileFormation, reactivity, photorelease, and scavenging of NO in ruthenium nitrosyl complexes, Product Details of C6H4N2, the main research area is pyridinyltriazinamine preparation reaction ruthenium complex; ruthenium pyridinyltriazinamine phenanthroline nitrosyl complex preparation crystal mol structure; nitrosyl photorelease ruthenium pyridinyltriazinamine phenanthroline complex.

The two newly designed nitrosyl complexes with Enemark-Feltham notation {RuNO}6 and {RuNO}7 configurations have been isolated as the perchlorate salts in the mol. framework [RuII(dmdptz)(phen)(NO)]n+ (dmdptz: N,N-dimethyl-4,6-di(pyridin-2-yl)-1,3,5-triazin-2-amine and phen: 1,10-phenanthroline) [RuII(dmdptz)(phen)(NO+)](ClO4)3 [4](ClO4)3 and [RuII(dmdptz)(phen)(NO·)](ClO4)2 [5](ClO4)2 resp. The single crystal x-ray structures of complexes [RuII(dmdptz)(phen)Cl](ClO4) [1](ClO4), [RuII(dmdptz)(phen)(NO2)](ClO4) [3](ClO4) and [4](ClO4)3 have been determined The π- acceptance of the NO+ moiety in [4](ClO4)3 is reflected from the triple bond characteristic bond length 1.131(5) Å with simultaneous trans angle of 175.3(4)° as a proof of true linear coordination mode. A sizable shift in ν(NO) frequency (Δν = 361 cm-1) on moving from [4](ClO4)3 to [5](ClO4)2 are in good agreement for largely NO centered reduction with the changes in bonding {RuNO}6 [4](ClO4)3 to {RuNO}7 [5](ClO4)2. The redox properties of [4](ClO4)3 along with the precursor complexes, have been investigated. On exposure to visible light in the deoxygenated acetonitrile solution at room temperature both [4](ClO4)3 and [5](ClO4)2 spontaneously transform to their corresponding solvated derivative [RuII(dmdptz)(phen)(CH3CN)](ClO4)2 [2](ClO4)2 via the facile photocleavage of Ru-NO bond with KNO 9.26 × 10-3 min-1 (t1/2 = 74 min) and 4.03 × 10-2 min-1 (t1/2 = 17 min) resp. The photoreleased “”NO”” can be scavenged by biol. relevant target mol. myoglobin as an Mb-NO adduct.

Inorganica Chimica Acta published new progress about Crystal structure. 100-70-9 belongs to class nitriles-buliding-blocks, name is Picolinonitrile, and the molecular formula is C6H4N2, Product Details of C6H4N2.

Referemce:
Nitrile – Wikipedia,
Nitriles – Chemistry LibreTexts